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  1. Topological defects are singularities in an ordered phase that can have a profound effect on phase transitions and serve as a window into the order parameter. Examples of topological defects include dislocations in charge density waves and vortices in a superconductor or pair density wave, where the latter is a condensate of Cooper pairs with finite momentum. Here we demonstrate the role of topological defects in the magnetic-field-induced disappearance of a charge density wave in the heavy-fermion superconductor UTe2. We reveal pairs of topological defects of the charge density wave with positive and negative phase winding. The pairs are directly correlated with zeros in the charge density wave amplitude and increase in number with increasing magnetic field. A magnetic field generates vortices of the superconducting and pair density wave orders that can create topological defects in the charge density wave and induce the experimentally observed melting of this charge order at the upper critical field. Our work reveals the important role of magnetic-field-generated topological defects in the melting of the charge density wave order parameter in UTe2 and provides support for the existence of a pair density wave order on the surface. 
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    Free, publicly-accessible full text available March 20, 2025
  2. The intense interest in triplet superconductivity partly stems from theoretical predictions of exotic excitations such as non-Abelian Majorana modes, chiral supercurrents and half-quantum vortices1–4. However, fundamentally new and unexpected states may emerge when triplet superconductivity appears in a strongly correlated system. Here we use scanning tunnelling microscopy to reveal an unusual charge-density-wave (CDW) order in the heavy-fermion triplet superconductor UTe2 (refs. 5–8). Our high-resolution maps reveal a multi-component incommensurate CDW whose intensity gets weaker with increasing field, with the CDW eventually disappearing at the superconducting critical field Hc2. To understand the phenomenology of this unusual CDW, we construct a Ginzburg–Landau theory for a uniform triplet superconductor coexisting with three triplet pair-density-wave states. This theory gives rise to daughter CDWs that would be sensitive to magnetic field owing to their origin in a pair-density-wave state and provides a possible explanation for our data. Our discovery of a CDW state that is sensitive to magnetic fields and strongly intertwined with superconductivity provides important information for understanding the order parameters of UTe2. 
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    Free, publicly-accessible full text available June 29, 2024
  3. Jelena Stajic (Ed.)

    Incorporating relativistic physics into quantum tunneling can lead to exotic behavior such as perfect transmission through Klein tunneling. Here, we probed the tunneling properties of spin-momentum-locked relativistic fermions by designing and implementing a tunneling geometry that uses nanowires of the topological Kondo insulator candidate samarium hexaboride. The nanowires are attached to the end of scanning tunneling microscope tips and used to image the bicollinear stripe spin order in the antiferromagnet Fe1.03Te with a Neel temperature of about 50 kelvin. The antiferromagnetic stripes become invisible above 10 kelvin concomitant with the suppression of the topological surface states in the tip. We further demonstrate that the direction of spin polarization is tied to the tunneling direction. Our technique establishes samarium hexaboride nanowires as ideal conduits for spin-polarized currents.

     
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  4. Spin chains in solid state materials are quintessential quantum systems with potential applications in spin-based logic, memory, quantum communication, and computation. A critical challenge is the experimental determination of spin lifetimes with the ultimate goal of increasing it. Local measurements by scanning tunneling microscopy (STM) have demonstrated the importance of decoupling spins from their environment, with markedly improved lifetimes in spin chains on the surfaces of band insulators. In this work we use low-temperature scanning tunneling microscopy to reveal long-lifetime excitations in a chain of spin-1/2 electrons embedded in a charge density wave Mott insulator, 1T-TaS 2 . Naturally occurring domain walls trap chains of localized spin-1/2 electrons in nearby sites, whose energies lie inside the Mott gap. Spin-polarized measurements on these sites show distinct two-level switching noise, as well as negative differential resistance in the dI/dV spectra, typically associated with spin fluctuations. The excitations show exceptionally long lifetimes of a few seconds at 300 mK. Our work suggests that layered Mott insulators in the chalcogenide family, which are amenable to exfoliation and lithography, may provide a viable platform for quantum applications. 
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  5. Abstract

    Higher order topological insulators (HOTIs) are a new class of topological materials which host protected states at the corners or hinges of a crystal. HOTIs provide an intriguing alternative platform for helical and chiral edge states and Majorana modes, but there are very few known materials in this class. Recent studies have proposed Bi as a potential HOTI, however, its topological classification is not yet well accepted. In this work, we show that the (110) facets of Bi and BiSb alloys can be used to unequivocally establish the topology of these systems. Bi and Bi0.92Sb0.08(110) films were grown on silicon substrates using molecular beam epitaxy and studied by scanning tunneling spectroscopy. The surfaces manifest rectangular islands which show localized hinge states on three out of the four edges, consistent with the theory for the HOTI phase. This establishes Bi and Bi0.92Sb0.08as HOTIs, and raises questions about the topological classification of the full family of BixSb1−xalloys.

     
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  6. Abstract

    The physical realization of Chern insulators is of fundamental and practical interest, as they are predicted to host the quantum anomalous Hall (QAH) effect and topologically protected chiral edge states which can carry dissipationless current. Current realizations of the QAH state often require complex heterostructures and sub-Kelvin temperatures, making the discovery of intrinsic, high temperature QAH systems of significant interest. In this work we show that time-reversal symmetry breaking Weyl semimetals, being essentially stacks of Chern insulators with inter-layer coupling, may provide a new platform for the higher temperature realization of robust chiral edge states. We present combined scanning tunneling spectroscopy and theoretical investigations of the magnetic Weyl semimetal, Co3Sn2S2. Using modeling and numerical simulations we find that depending on the strength of the interlayer coupling, chiral edge states can be localized on partially exposed kagome planes on the surfaces of a Weyl semimetal. Correspondingly, our dI/dVmaps on the kagome Co3Sn terraces show topological states confined to the edges which display linear dispersion. This work provides a new paradigm for realizing chiral edge modes and provides a pathway for the realization of higher temperature QAH effect in magnetic Weyl systems in the two-dimensional limit.

     
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  7. null (Ed.)
  8. The possible realization of Majorana fermions as quasiparticle excitations in condensed-matter physics has created much excitement. Most studies have focused on Majorana bound states; however, propagating Majorana states with linear dispersion have also been predicted. Here, we report scanning tunneling spectroscopic measurements of crystalline domain walls (DWs) in FeSe 0.45 Te 0.55 . We located DWs across which the lattice structure shifts by half a unit cell. These DWs have a finite, flat density of states inside the superconducting gap, which is a hallmark of linearly dispersing modes in one dimension. This signature is absent in DWs in the related superconductor, FeSe, which is not in the topological phase. Our combined data are consistent with the observation of dispersing Majorana states at a π-phase shift DW in a proximitized topological material. 
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  9. Abstract

    The path from a Mott insulating phase to high temperature superconductivity encounters a rich set of unconventional phenomena involving the insulator-to-metal transition (IMT), such as emergent electronic orders and pseudogaps, that ultimately affect the condensation of Cooper pairs. A huge hindrance to understanding the origin of these phenomena is the difficulty in accessing doping levels near the parent state. TheJeff = 1/2 Mott state of the perovskite strontium iridates has revealed intriguing parallels to the cuprates, with the advantage that it provides unique access to the Mott transition. Here, we exploit this accessibility to study the IMT and the possible nearby electronic orders in the electron-doped bilayer iridate (Sr1 − xLax)3Ir2O7. Using spectroscopic imaging scanning tunneling microscopy, we image the La dopants in the top as well as the interlayer SrO planes. Surprisingly, we find a disproportionate distribution of La between these layers with the interlayer La being primarily responsible for the IMT. This reveals the distinct site-dependent effects of dopants on the electronic properties of bilayer systems. Electron doping also results in charge reordering. We find unidirectional electronic order concomitant with the structural distortion known to exist in this system. Intriguingly, similar to the single layer iridate, we also find local resonant states forming a checkerboard-like pattern trapped by La. This suggests that multiple charge orders may exist simultaneously in Mott systems, even with only one band crossing the Fermi energy.

     
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